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dc.contributor.authorMichaud, Alexander B.
dc.contributor.authorDore, John E.
dc.contributor.authorPriscu, John C.
dc.contributor.authorLeslie, Deborah
dc.contributor.authorLyons, W. Berry
dc.contributor.authorSands, David C.
dc.date.accessioned2015-03-06T20:22:19Z
dc.date.available2015-03-06T20:22:19Z
dc.date.issued2014-11
dc.identifier.citationMichaud, Alexander B., John E. Dore, John C. Priscu, Deborah Leslie, W. Berry Lyons, and David C. Sands. "Biological ice nucleation initiates hailstone formation." Journal of Geophysical Research: Atmospheres (2014).http://dx.doi.org/10.1002/2014JD022004en_US
dc.identifier.issn2169-897X
dc.identifier.urihttp://dx.doi.org/10.1002/2014JD022004
dc.identifier.urihttps://scholarworks.montana.edu/xmlui/handle/1/8920
dc.description.abstractCloud condensation and ice nuclei in the troposphere are required precursors to cloud and precipitation formation, both of which influence the radiative balance of Earth. The initial stage of hailstone formation (i.e., the embryo) and the subsequent layered growth allow hail to be used as a model for the study of nucleation processes in precipitation. By virtue of the preserved particle and isotopic record captured by hailstones, they represent a unique form of precipitation that allows direct characterization of the particles present during atmospheric ice nucleation. Despite the ecological and economic consequences of hail storms, the dynamics of hailstone nucleation, and thus their formation, are not well understood. Our experiments show that hailstone embryos from three Rocky Mountain storms contained biological ice nuclei capable of freezing water at warm, subzero (°C) temperatures, indicating that biological particles can act as nucleation sites for hailstone formation. These results are corroborated by analysis of δD and δ18O from melted hailstone embryos, which show that the hailstones formed at similarly warm temperatures in situ. Low densities of ice nucleation active abiotic particles were also present in hailstone embryos, but their low concentration indicates they were not likely to have catalyzed ice formation at the warm temperatures determined from water stable isotope analysis. Our study provides new data on ice nucleation occurring at the bottom of clouds, an atmospheric region whose processes are critical to global climate models but which has challenged instrument-based measurements.en_US
dc.subjectAtmospheric sciencesen_US
dc.subjectChemistryen_US
dc.titleBiological ice nucleation initiates hailstone formationen_US
dc.typeArticleen_US
mus.citation.extentfirstpage12186en_US
mus.citation.extentlastpage12197en_US
mus.citation.issue21en_US
mus.citation.journaltitleJournal of Geophysical Research: Atmospheresen_US
mus.citation.volume119en_US
mus.identifier.categoryLife Sciences & Earth Sciencesen_US
mus.identifier.doi10.1002/2014JD022004en_US
mus.relation.collegeCollege of Agricultureen_US
mus.relation.collegeCollege of Agriculture
mus.relation.departmentLand Resources & Environmental Sciences.en_US
mus.relation.departmentPlant Sciences & Plant Pathology.en_US
mus.relation.universityMontana State University - Bozemanen_US
mus.contributor.orcidSands, David C.|0000-0002-3749-2817en_US


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