Theses and Dissertations at Montana State University (MSU)
Permanent URI for this collectionhttps://scholarworks.montana.edu/handle/1/733
Browse
3 results
Search Results
Item Thermalization and exciton localization in 2D semiconductors(Montana State University - Bozeman, College of Letters & Science, 2023) Strasbourg, Matthew Christopher; Chairperson, Graduate Committee: Nick Borys; This is a manuscript style paper that includes co-authored chapters.2D semiconductors are a promising class of materials to investigate for applications in the next generation of photonic devices. They can be used to generate quantum light and also exhibit correlated many-body phenomena. Many of the novel optoelectronic properties of 2D semiconductors are associated with strongly-bound hydrogen-like states known as excitons. Excitons in 2D semiconductors have binding energies on the order of 100s of meV and are stable at room temperature. At low temperatures, higher-order excitonic states such as charged excitons and biexcitons--multiple-bound excitons that are like hydrogen molecules-- and localized excitons that emit quantum light are also observed. Whether excited optically or electronically, a diversity of high-energy excitons and free carriers are produced directly after excitation. The relaxation and thermalization of these initial states influence the formation of excitons, biexcitons, and localized excitons. Here, I present work that (i) investigates the thermalization of excited states in a prototypical 2D semiconductor, monolayer (1L-) WSe2, and reports the discovery that the generation of charged biexcitons is enhanced with increasing photoexcitation energy, (ii) shows the emergence of quantum emitters (QEs) in a new 2D QE platform: 1L-WSe2 nanowrinkle arrays induced by Au nano stressors, and (iii) uses a novel method to classify the excited-state dynamics of 2D QEs and differentiate emitter populations. A suite of low-temperature energy- and time- resolved optical spectroscopies are used to conduct this work. This work shows how excited state thermalization affects the formation of exciton and biexcitons and investigates the optical properties of an emergent class of 2D quantum light emitters.Item Theoretical analysis and experimental design of dual-beam optical trap for large particles(Montana State University - Bozeman, College of Letters & Science, 2018) St. John, Demi Rose; Chairperson, Graduate Committee: Wm. Randall BabbittUltra-high sensitivity acceleration and gryometric sensors have been proposed as optically levitated particles in ultra-high vacuum (UHV). Larger particles (10- 30 microns in diameter) provide higher sensitivity, but they are difficult to trap in UHV without particle loss. To overcome the radiometric forces that lead to particle loss, rare earth (RE) ion dopants can be incorporated into the particles to enable solid-state laser cooling of the particles internal temperature. This thesis theoretically and experimentally explores development of optical traps designed for trapping and internally laser cooling large particles. The analysis focuses on dual-beam horizontal traps and the development of code to analyze dual-beam trap potentials and particle loading dynamics. Tolerance analysis, improved particle loader designs, and monitoring and automation of the loading process are investigated. The thesis provides a road map for achieving efficient optical trapping, cooling, and control of large particles.Item Demonstration of normalized differential detection using smart pixels with smart illumination(Montana State University - Bozeman, College of Letters & Science, 2000) Chen, Xiaofang