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Item Water Vapor Profiling using a Widely Tunable, Amplified Diode Laser Based Differential Absorption Lidar (DIAL)(2009-04) Nehrir, Amin R.; Repasky, Kevin S.; Carlsten, John L.; Obland, Michael D.; Shaw, Joseph A.A differential absorption lidar (DIAL) instrument for automated profiling of water vapor in the lower troposphere has been designed, tested, and is in routine operation at Montana State University. The laser transmitter for the DIAL instrument uses a widely tunable external cavity diode laser (ECDL) to injection seed two cascaded semiconductor optical amplifiers (SOAs) to produce a laser transmitter that accesses the 824–841-nm spectral range. The DIAL receiver utilizes a 28-cm-diameter Schmidt–Cassegrain telescope; an avalanche photodiode (APD) detector; and a narrowband optical filter to collect, discriminate, and measure the scattered light. A technique of correcting for the wavelength-dependent incident angle upon the narrowband optical filter as a function of range has been developed to allow accurate water vapor profiles to be measured down to 225 m above the surface. Data comparisons using the DIAL instrument and collocated radiosonde measurements are presented demonstrating the capabilities of the DIAL instrument.Item Observational Studies of Atmospheric Aerosols over Bozeman, Montana, Using a Two-Color Lidar, a Water Vapor DIAL, a Solar Radiometer, and a Ground-Based Nephelometer over a 24-h Period(2011-03) Repasky, Kevin S.; Reagan, John A.; Nehrir, Amin R.; Hoffman, David S.; Thomas, Michael J.; Carlsten, John L.; Shaw, Joseph A.; Shaw, Glenn E.Coordinated observational data of atmospheric aerosols were collected over a 24-h period between 2300 mountain daylight time (MDT) on 27 August 2009 and 2300 MDT on 28 August 2009 at Bozeman, Montana (45.66°N, 111.04°W, elevation 1530 m) using a collocated two-color lidar, a diode-laser-based water vapor differential absorption lidar (DIAL), a solar radiometer, and a ground-based nephelometer. The optical properties and spatial distribution of the atmospheric aerosols were inferred from the observational data collected using the collocated instruments as part of a closure experiment under dry conditions with a relative humidity below 60%. The aerosol lidar ratio and aerosol optical depth retrieved at 532 and 1064 nm using the two-color lidar and solar radiometer agreed with one another to within their individual uncertainties while the scattering component of the aerosol extinction measured using the nephelometer matched the scattering component of the aerosol extinction retrieved using the 532-nm channel of the two-color lidar and the single-scatter albedo retrieved using the solar radiometer. Using existing aerosol models developed with Aerosol Robotic Network (AERONET) data, a thin aerosol layer observed over Bozeman was most likely identified as smoke from forest fires burning in California; Washington; British Columbia, Canada; and northwestern Montana. The intrusion of the thin aerosol layer caused a change in the atmospheric radiative forcing by a factor of 1.8 ± 0.5 due to the aerosol direct effect.Item Eye-Safe Diode-Laser-Based Micropulse Differential Absorption Lidar (DIAL) for Water Vapor Profiling in the Lower Troposphere(2011-02) Nehrir, Amin R.; Repasky, Kevin S.; Carlsten, John L.A second-generation diode-laser-based master oscillator power amplifier (MOPA) configured micropulse differential absorption lidar (DIAL) instrument for profiling of lower-tropospheric water vapor is presented. The DIAL transmitter is based on a continuous wave (cw) external cavity diode laser (ECDL) master oscillator that is used to injection seed two cascaded tapered semiconductor optical power amplifiers, which deliver up to 2-μJ pulse energies over a 1-μs pulse duration at 830 nm with an average power of ∼40 mW at a pulse repetition frequency of 20 kHz. The DIAL receiver utilizes a commercial 28-cm-diameter Schmidt–Cassegrain telescope, a 250-pm narrowband optical filter, and a fiber-coupled single-photon-counting Avalanche photodiode (APD) detector, yielding a far-field full-angle field of view of 170 μrad. A detailed description of the second-generation Montana State University (MSU) DIAL instrument is presented. Water vapor number density profiles and time–height cross sections collected with the water vapor DIAL instrument are also presented and compared with collocated radiosonde measurements, demonstrating the instruments ability to measure night- and daytime water vapor profiles in the lower troposphere.Item Optical Characterization of Continental and Biomass Burning Aerosols over Bozeman Montana: A Case Study of the Aerosol Direct Effect(2011-11) Nehrir, Amin R.; Repasky, Kevin S.; Reagan, John A.; Carlsten, John L.Atmospheric aerosol optical properties were observed from 21 to 27 September 2009 over Bozeman, Montana, during a transitional period in which background polluted rural continental aerosols and well‐aged biomass‐burning aerosols were the dominant aerosol types of extremely fresh biomass‐burning aerosols resulting from forest fires burning in the northwestern United States and Canada. Aerosol optical properties and relative humidity profiles were retrieved using an eye‐safe micropulse water vapor differential absorption lidar (DIAL) (MP‐DIAL), a single‐channel backscatter lidar, a CIMEL solar radiometer as part of the Aerosol Robotic Network (AERONET), a ground‐based integrating nephelometer, and aerosol products from Moderate Resolution Imaging Spectroradiometer (MODIS) Terra and Aqua. Aerosol optical depths (AODs) measured during the case study ranged between 0.03 and 0.17 (0.015 and 0.075) at 532 nm (830 nm) as episodic combinations of fresh and aged biomass‐burning aerosols dominated the optical depth of the pristinely clean background air. Here, a pristinely clean background refers to very low AOD conditions, not that the aerosol scattering and absorption properties are necessarily representative of a clean aerosol type. Diurnal variability in the aerosol extinction to backscatter ratio (Sa) of the background atmosphere derived from the two lidars, which ranged between 55 and 95 sr (50 and 90 sr) at 532 nm (830 nm), showed good agreement with retrievals from AERONET sun and sky measurements over the same time period but were consistently higher than some aerosol models had predicted. Sa measured during the episodic smoke events ranged on average from 60 to 80 sr (50 to 70 sr) at 532 nm (830 nm) while the very fresh biomass‐burning aerosols were shown to exhibit significantly lower Sa ranging between 20 and 40 sr. The shortwave direct radiative forcing that was due to the intrusion of biomass‐burning aerosols was calculated to be on average −10 W/m2 and was shown to compare favorably with regional‐scale forcing calculations using MODIS‐Terra and AERONET data in an effort to assess the accuracy of estimating the regional‐scale aerosol direct radiative forcing effect using aerosol optical properties measured from a single rural site such as Bozeman, Montana.Item Micropulse Water Vapor Differential Absorption Lidar: Transmitter Design and Performance(2012-10) Nehrir, Amin R.; Repasky, Kevin S.; Carlsten, John L.An all diode-laser-based micropulse differential absorption lidar (DIAL) laser transmitter for tropospheric water vapor and aerosol profiling is presented. The micropulse DIAL (MPD) transmitter utilizes two continuous wave (cw) external cavity diode lasers (ECDL) to seed an actively pulsed, overdriven tapered semiconductor optical amplifier (TSOA). The MPD laser produces up to 7 watts of peak power over a 1 µs pulse duration (7 µJ) and a 10 kHz pulse repetition frequency. Spectral switching between the online and offline seed lasers is achieved on a 1Hz basis using a fiber optic switch to allow for more accurate sampling of the atmospheric volume between the online and offline laser shots. The high laser spectral purity of greater than 0.9996 coupled with the broad tunability of the laser transmitter will allow for accurate measurements of tropospheric water vapor in a wide range of geographic locations under varying atmospheric conditions. This paper describes the design and performance characteristics of a third generation MPD laser transmitter with enhanced laser performance over the previous generation DIAL system.Item Field demonstration of a 1 x 4 Fiber Sensor Array for Sub-Surface Carbon Dioxide Monitoring for Carbon Sequestration(2014-01) Soukup, Benjamin J.; Repasky, Kevin S.; Carlsten, John L.; Wicks, Geoffrey R.A fiber sensor array for subsurface CO 2 concentration measurements was developed for monitoring geologic carbon sequestration sites. The fiber sensor array uses a single temperature-tunable distributed feedback (DFB) laser operating with a nominal wavelength of 2.004 μm. Light from this DFB laser is directed to one of the four probes via an inline 1×4 fiber optic switch. Each of the four probes is buried and allows the subsurface CO 2 to enter the probe through Millipore filters that allow the soil gas to enter the probe but keeps out the soil and water. Light from the DFB laser interacts with the CO 2 before it is directed back through the inline fiber optic switch. The DFB laser is tuned across two CO 2 absorption features, where a transmission measurement is made allowing the CO 2 concentration to be retrieved. The fiber optic switch then directs the light to the next probe where this process is repeated, allowing subsurface CO 2 concentration measurements at each of the probes to be made as a function of time. The fiber sensor array was deployed for 58 days beginning from June 19, 2012 at the Zero Emission Research Technology field site, where subsurface CO 2 concentrations were monitored. Background measurements indicate that the fiber sensor array can monitor background levels as low as 1000 parts per million (ppm). A 34-day subsurface release of 0.15 tones CO 2 /day began on July 10, 2012. The elevated subsurface CO 2 concentration was easily detected by each of the four probes with values ranging over 60,000 ppm, a factor of greater than 6 higher than background measurements.